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A New Entry of Amination Reagents for Heteroaromatic C–H Bonds: Copper-Catalyzed Direct Amination of Azoles with Chloroamines at
Over the last decade, transition-metal-mediated or -catalyzed reactions involving a C–H bond cleavage have received much attention and the area has grown rapidly because of the possibility of transforming ubiquitous C–H bonds into versatile functions in just one synthetic step. In 1997, Professor Masahiro Miura and co-workers from Osaka University (Japan) reported the palladium-catalyzed direct arylation of phenolic compounds with aryl halides (Angew. Chem., Int. Ed. Engl. 1997, 36, 1740), which is one of the pioneering works in the field of C–H bond activation chemistry.
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